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By Ji-Xin Cheng, Xiaoliang Sunney Xie

Conception idea of Coherent Raman Scattering, Eric Olaf Potma and Shaul MukamelCoherent Raman Scattering less than Tightly targeted stipulations, Eric Olaf Potma, Xiaoliang Sunney Xie, Andreas Volkmer, and Ji-Xin ChengPlatformsConstruction of a Coherent Raman Microscope, Brian G. Sarr and Xiaoliang Sunney XieStimulated Raman Scattering Microscopy, Christian Freudiger and Xiaoliang Sunney XieFemtosecond as opposed to Picosecond Read more...

summary: conception thought of Coherent Raman Scattering, Eric Olaf Potma and Shaul MukamelCoherent Raman Scattering below Tightly centred stipulations, Eric Olaf Potma, Xiaoliang Sunney Xie, Andreas Volkmer, and Ji-Xin ChengPlatformsConstruction of a Coherent Raman Microscope, Brian G. Sarr and Xiaoliang Sunney XieStimulated Raman Scattering Microscopy, Christian Freudiger and Xiaoliang Sunney XieFemtosecond as opposed to Picosecond Pulses for Coherent Raman Microscopy, Mikhail N. Slipchenko, Delong Zhang, and Ji-Xin ChengWide-Field automobiles Microscopy, Alexander Jesacher, Gregor Thalhammer, Stefan Bernet, and Monika R

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1 Electronic and Nuclear Motions Although it is the electrons in the molecule that are set in motion by the visible or near-IR driving fields, their oscillatory motions do contain information about the motions of nuclei. The reason for this is that the adiabatic electronic potential depends on the nuclear coordinates. Since the electrons are bound to the nuclei, Theory of Coherent Raman Scatterin 11 nuclear motions will affect the motions of the electrons as well. Hence, the electronic polarizability is perturbed by the presence of nuclear modes.

Therefore, a better classification for SRL and SRG techniques would be Raman sensitive pump-probe, which more accurately captures the nature of the detected signal. 2), but the reader is warned about the existing ambiguities in the current nomenclature. 1 Electronic and Nuclear Motions Although it is the electrons in the molecule that are set in motion by the visible or near-IR driving fields, their oscillatory motions do contain information about the motions of nuclei. The reason for this is that the adiabatic electronic potential depends on the nuclear coordinates.

In the SRG channel this interference is constructive, producing a gain of the overall ω2 field, whereas in the SRL channel the interference is destructive, giving rise to a loss of the amplitude of the ω1 field. The extend of the loss and gain scales with Im{χNL}, which describes the dissipative part of the interaction. 6 Semi-Classical Description: Quantum Matter and Classical Fields The fully classical model provides a qualitative description of the coherent Raman process in which the nuclear motion is described as a harmonic oscillator.

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