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G. G. Ertl: Proc. Solvay Conf. on Surface Science, ed. W. De Wette (Springer, Berlin, Heidelberg 1988), p. 322 I. Langmuir, Trans. Faraday Soc. 17 (1922), 621 M. Bodenstein, F. OhImer: Z. Phys. Chern. 53 (1905), 166 M. G. Fink: Z. Phys. Chern. 60 (1907), 1 G. Ertl, P. Rau: Surface Sci. 15 (1969), 443 T. Engel, G. Ertl: Adv. Catalysis 28 (1979), 1 T. Engel, G. Enl: J. Chern. Phys. T. Campbell, G. Ertl, H. Kuipers, J. Segner: J. Chern. Phys. 73 (1980),5862 G. Enl: In Chemistry and Physics of Solid Surfaces Ill, ed.

A. Trevino, to be published M. Boudan, to be published S. Ladas, R. Imbihl, G. : Surface Sci. 197 (1988), 153 M. D. Schmidt: Progr. Surf. Sci. 92 22 R. E. Reynolds, D. Kaletta, to be published O. Ertl, Adv. Catalysis 37 (1990), in press G. Nicolis, I. M. Turing: Phil. Trans. Roy. Soc. (London) B 237 (1952), 37 M. Eiswirth, O. Ertl: Surf. Sci. 177 (1986), 90 P. Hugo: Ber. Bunsenges. Phys. Chern. 74 (1970), 121; H. Beusch, P. Fieguth, E. Wicke: Chern. Ing. Techn. F. A. Schmitz: Catal. Rev. 28 (1986), 89; Chern.

R: III en Z w 10 ! 5 o L-__~____~____~__~~__~ 460 820 100 TEMPERATURE (K) methyl fragments are hydrogenated using hydrogen either accumulated from the background or from a modest decomposition of CH3 itself. There is an interesting contrast with Ag{ 111}; the exclusive C- and H-containing product is ethane. Armed with these results, we substantiated this interpretation through: (1) HREELS measurements which identify the CH3 group bound to the Pt through a C-Pt bond, the presence of a strong Br-Pt bond, and the absence of C-Br bonds, when the parent molecules are desorbed and (2) XPS measurements which distinguish the Br in CH3Br from that in Pt-Br on the basis of a I eV core level binding energy shift, and which demonstrate that some parent is thermally desorbed, not photo-desorbed.

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